Swiss Nanoscience Institute Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung. Grant Number: Sinergia CRSII5_202296 Rutherford Appleton Laboratory Faraday Institution alloy interlayer | all-solid-state battery | image subtraction method | Li metal | operando XCT | zero-excess lithium anode

Xu, Linfeng, Le Houx, James ORCID: https://orcid.org/0000-0002-1576-0673, Kachkanov, Vyacheslav, Zhang, Jinsong, Norbert Wullich, Robin, Fankhauser, Matthias, Löffel, Kaspar, Schmidt, Thomas J. and El Kazzi, Mario (2026) Operando X‐Ray computed tomography reveals the role of interfacial nucleation nanolayers in suppressing mechanical failure in zero‐excess lithium all‐solid‐state batteries. Small:e12284. ISSN 1613-6810 (Print), 1613-6829 (Online) (doi:10.1002/smll.202512284)

autonomous experimentation, large-scale user facilities, AI for science, taxonomy, Operational Design Domains (ODD), sim-to-real transfer

Le Houx, James ORCID: https://orcid.org/0000-0002-1576-0673 (2026) Benchmarking autonomy in scientific experiments: a hierarchical taxonomy for autonomous large-scale facilities. [Working Paper] (doi:10.48550/arXiv.2601.06978)

autonomous experimentation, operando characterisation, battery degradation, scientific AI, physics,. informed machine learning

Lu, Emily, Perez, Gabriel, Baker, Peter, Irving, Daniel, Kumar, Santosh, Celorrio, Veronica, Britto, Sylvia, Headen, Thomas F., Gomez-Gonzalez, Miguel, Wright, Connor, Green, Calum, Young, Robert Scott, Kirichek, Oleg, Mortazavi, Ali, Day, Sarah, Antony, Isabel, Wright, Zoe, Wood, Thomas, Snow, Tim, Thiyagalingam, Jeyan, Quinn, Paul, Jones, Martin Owen, David, William and Le Houx, James ORCID: https://orcid.org/0000-0002-1576-0673 (2026) Autonomous battery research: principles of heuristic operando experimentation. [Working Paper] (doi:10.48550/arxiv.2601.00851)